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Entangled photon pairs are a crucial resource in quantum information processing. However, common sources of entangled photon pairs, such as generation by spontaneous parametric down-conversion, impose a Poisson distribution on the pairs, limiting their applicability to quantum information processing. Therefore, generating entangled photon pairs exhibiting a sub-Poisson distribution (i.e., entangled photon bundle) would be crucial/an important advancement in the current research context. Recently, it has been proposed that antibunched photon pairs can be generated using pulsed excitation of quantum dots based on photon blockade. In this work we propose a scheme to generate entangled photon pairs with strong antibunching properties via continuous driving. Under two-photon resonant continuous pumping, a quantum dot is first excited to a biexciton state and then emits a pair of entangled photons into a two-mode cavity. Owing to the strong coupling between the quantum dot and optical modes of the cavity, at most one pair of left-/right-polarized photons exists at a time in the cavity. Specifically, the antibunching effect, average photon number, and entanglement of the left- or right-polarized photons can be resonantly enhanced when the coupling strengths between the exciton (biexciton) transition and cavity modes are equal. Moreover, our results show that the binding energy of the biexciton substantially affects the antibunching effect, average photon number, and entanglement of the left-/right-polarized photons. With suitable parameters, we can realize photon pairs with strong antibunching, a large average photon number, and deep entanglement. Hence, the studied quantum dot-cavity system is a promising source of antibunched entangled photon pairs.
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http://dx.doi.org/10.1364/OE.567201 | DOI Listing |
Phys Rev Lett
August 2025
Universität Innsbruck, Institut für Experimentalphysik, Technikerstrasse 25, 6020 Innsbruck, Austria.
Establishing networks of quantum processors offers a path to scalable quantum computing and applications in communication and sensing. This requires first developing efficient interfaces between photons and multiqubit registers. In this Letter, we show how to entangle each individual matter qubit in a register of ten to a separate traveling photon.
View Article and Find Full Text PDFLight Sci Appl
September 2025
Laboratory of Quantum Information, University of Science and Technology of China, 230026, Hefei, China.
Quantum imaging with spatially entangled photons offers advantages such as enhanced spatial resolution, robustness against noise, and counterintuitive phenomena, while a biphoton spatial aberration generally degrades its performance. Biphoton aberration correction has been achieved by using classical beams to detect the aberration source or scanning the correction phase on biphotons if the source is unreachable. Here, a new method named position-correlated biphoton Shack-Hartmann wavefront sensing is introduced, where the phase pattern added on photon pairs with a strong position correlation is reconstructed from their position centroid distribution at the back focal plane of a microlens array.
View Article and Find Full Text PDFNat Photonics
June 2025
University of Vienna, Faculty of Physics, Vienna Center for Quantum Science and Technology (VCQ), Vienna, Austria.
Recently, machine learning has had remarkable impact in scientific to everyday-life applications. However, complex tasks often require the consumption of unfeasible amounts of energy and computational power. Quantum computation may lower such requirements, although it is unclear whether enhancements are reachable with current technologies.
View Article and Find Full Text PDFNanoscale Horiz
September 2025
Theoretical Chemical Physics Group, Research Institute for Materials Science and Engineering, University of Mons, 20 Place du Parc, Mons B-7000, Belgium.
Two-photon spontaneous emission (TPSE) is a second-order quantum process with promising applications in quantum optics that remains largely unexplored in molecular systems, which are usually very inefficient emitters. In this work, we model the first molecular two-photon emitters and establish the design rules, highlighting their differences from those governing two-photon absorbers. Using both time-dependent density functional theory and Pariser-Parr-Pople calculations, we calculate TPSE in three π-conjugated molecules and identify a dominant pathway.
View Article and Find Full Text PDFAdv Mater
September 2025
School of Chemistry and Biochemistry, School of Materials Science and Engineering, Center for Organic Photonics and Electronics, Georgia Institute of Technology, Atlanta, GA, 30332, USA.
Molecular spin systems that can be chemically tuned, coherently controlled, and readily integrated within devices remain central to the realization of emerging quantum technologies. Organic high-spin materials are prime candidates owing to their similarity in electronic structure to leading solid-state defect-based systems, light element composition, and the potential for entanglement and qubit operations mediated through spin-spin exchange. However, the inherent instability of these species precludes their rational design, development, and application.
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