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Article Abstract

Polarization photodetectors suffer from insufficient sensitivity, slow response speed, and limited spectral response range. Therefore, the development of new photodetectors with broad spectral response, high sensitivity, excellent polarization sensitivity, and low cost has become the focus of the current research field. Herein, we report an InSe/CIPS heterojunction-based approach for high-performance photodetection, polarization-sensitive photodetection, and polarization imaging in the visible to near-infrared region (400-808 nm). Its high responsivity (41.42 A/W at 532 nm and 18.95 A/W at 808 nm) and specific detectivity (9.79 × 10 Jones at 532 nm and 4.51 × 10 Jones at 808 nm) outperforms most two-dimensional heterojunction photodetectors. In addition, the heterojunction has a fast response time (0.17/0.33 s at 400 nm) and broadband polarization detection (6.04 at 400 nm and 5.7 at 808 nm). The proposed hierarchical fusion strategy effectively coordinates the multiangle polarization information, improves the response of polarization imaging detectors to signals under complex optical fields, and provides an effective image processing framework to enhance the environmental adaptability of polarization detectors, which further promotes the application of polarization detectors in high-precision photoelectric detection.

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http://dx.doi.org/10.1021/acsami.5c07538DOI Listing

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