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Owing to the growing demand for scaling down and low-power consumption in the Internet of Things and wearable devices, there is an increasing need for miniaturized, self-powered flexible optoelectronics with omnidirectional photodetection ability. In this work, a mixed-dimensional heterojunction near-ultraviolet photodetector of CdS nanobelts/PbI nanosheets was prepared chemical vapor deposition and liquid-phase growth methods. Importantly, the as-fabricated self-powered near-ultraviolet photodetector displayed a low of 7 × 10 A, high / ratio of 2.06 × 10, fast rise/decay times of 581 μs/581 μs and exceptional responsivity and detectivity of 3446.04 mA W and 9.05 × 10 Jones, respectively, benefiting from the built-in field. In addition, the flexible near-ultraviolet photodetector exhibited impressive omnidirectional photodetection and robust bending endurance. Thus, all these results reveal the technological potential of the mixed-dimensional photodetector for next-generation high-performance near-ultraviolet optoelectronics.
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http://dx.doi.org/10.1039/d5nr00712g | DOI Listing |
Phys Chem Chem Phys
August 2025
School of Information Engineering, Jiangxi University of Science and Technology, Ganzhou 341000, China.
Two-dimensional (2D) heterostructure materials, known for their tunable multifunctionality and low-dimensional confinement effects, offer vast potential for diverse applications. This work provides a comprehensive investigation of the electronic structure, transport and optical properties of MoSe/ZrCl heterostructures using density functional theory (DFT) with non-equilibrium Green's function (NEGF) methods. Our results demonstrate that the electronic properties of MoSe/ZrCl heterostructure materials can be precisely tuned by applying biaxial strain.
View Article and Find Full Text PDFPhotoresponse waveforms visually describe the charge carrier dynamics in a photodetector (PD) and serve as a means of conveying optical information, analogous to the photoresponse amplitude and polarity. Nevertheless, the waveforms of most photodetectors are frequently neglected due to the difficulty of distinguishing them. Herein, three distinct waveform modes are realized in a self-powered n-Si/Au nanoparticle/CdS heterojunction photodetector, corresponding to different wavelengths from the near-ultraviolet to near-infrared spectrum.
View Article and Find Full Text PDFNanoscale
May 2025
School of Physics, State Key Laboratory of Crystal Materials, Shandong University, Jinan, 250100, China.
Owing to the growing demand for scaling down and low-power consumption in the Internet of Things and wearable devices, there is an increasing need for miniaturized, self-powered flexible optoelectronics with omnidirectional photodetection ability. In this work, a mixed-dimensional heterojunction near-ultraviolet photodetector of CdS nanobelts/PbI nanosheets was prepared chemical vapor deposition and liquid-phase growth methods. Importantly, the as-fabricated self-powered near-ultraviolet photodetector displayed a low of 7 × 10 A, high / ratio of 2.
View Article and Find Full Text PDFSmall
February 2025
School of Microelectronics, Northwestern Polytechnical University, 127 West Youyi Road, Beilin District, Xi'an, Shaanxi, 710072, P. R. China.
Nanotechnology
December 2024
Universidad de Chile, Blanco Encalada 2008, Santiago de Chile, 1025000, CHILE.
Graphene has garnered significant interest in optoelectronics due to its unique properties, including broad wavelength absorption and high mobility. However, its weak stability in ambient conditions requires encapsulation for practical applications. In this study, we investigate graphene CVD-grown field-effect transistors fabricated on Si/SiOwafers, encapsulated with aluminum oxide (AlO) of different thicknesses.
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