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Hole-doped cuprates exhibit partially coexisting pseudogap (PG), charge ordering (CO) and superconductivity; we show that there exists a class of systems in which they have a single nature as it has recently been supposed. Since the charge-ordered phase exhibits large frozen deformation of the lattice, we develop a method for calculating the phase diagram of a system with strong long-range (Fröhlich) electron-phonon interaction. Using a variational approach, we calculate the free energy of a two-liquid system of carriers with cuprate-like dispersion comprising a liquid of autolocalized carriers (large polarons and bipolarons) and Fermi liquid of delocalized carriers. Comparing it with the free energy of pure Fermi liquid and calculating (with standard methods of Bose liquid theory) a temperature of the superfluid transition in the large-bipolaron liquid we identify regions in the phase diagram with the presence of PG (caused by the impact of the (bi)polarons potential on delocalized quasiparticles), CO and superconductivity. They are located in the same places in the diagram as in hole-doped cuprates, and, as in the latter, the shape of the calculated phase diagram is resistant to wide-range changes in the characteristics of the system. As in cuprates, the calculated temperature of the superconducting transition increases with the number of conducting planes in the unit cell, the superfluid density decreases with doping at overdoping, the bipolaron density (and bipolaronic plasmon energy) saturates at optimal doping. Thus, the similarity of the considered system with hole-doped cuprates is not limited to the phase diagram. The results obtained allow us to discuss ways of increasing the temperature of the superfluid transition in the large-bipolaron liquid and open up the possibility of studying the current-carrying state and properties of the bipolaron condensate.
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http://dx.doi.org/10.1088/1361-648X/ad459d | DOI Listing |
Nano Lett
June 2025
Beijing National Laboratory for Condensed Matter Physics and Institute of Physics, Chinese Academy of Sciences, Beijing 100190, China.
Landau's Fermi liquid theory offers a profound understanding of conduction electrons in metals. However, many strongly correlated materials, including heavy-fermions, cuprates, iron-based superconductors, and nickelates, exhibit non-Fermi liquid (NFL) behavior. A hallmark is the strange metal state, characterized by linear-in-temperature resistivity and a linear-in-energy single-particle decay rate.
View Article and Find Full Text PDFProc Natl Acad Sci U S A
May 2025
Department of Physics and Quantum Centre of Excellence for Diamond and Emergent Materials, Indian Institute of Technology Madras, Chennai 600036, India.
We employ a family of ancilla qubit variational wave functions [Y.-H. Zhang and S.
View Article and Find Full Text PDFPhys Rev Lett
March 2025
Ludwig-Maximilians-Universität München, Arnold Sommerfeld Center for Theoretical Physics, 80333 Munich, Germany.
The two-dimensional Hubbard model is widely believed to capture key ingredients of high-T_{c} superconductivity in cuprate materials. However, compelling evidence remains elusive. In particular, various magnetic orders may emerge as strong competitors of superconducting orders.
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