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Unidirectional and long-distance liquid transport is critically important to a range of practical applications, e.g., water harvesting, microfluidics, and chemical reactions. Great efforts have been made on liquid manipulation; most of which, however, are limited in the air environment. It is still a great challenge to achieve unidirectional and long-distance oil transport in an aqueous environment. Herein, we have successfully fabricated an underwater superoleophilic two-dimensional surface (USTS) with asymmetric oleophobic barriers to arbitrarily manipulate oil in aqueous medium. The behavior of oil on USTS was carefully investigated, of which the unidirectional spreading capability was originated from the anisotropic spreading resistance resulted from the asymmetric oleophobic barriers. Accordingly, an underwater oil/water separation device has been developed, which can achieve continuous and efficient oil/water separation and further prevent the secondary pollution caused by oil volatilization.
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http://dx.doi.org/10.1021/acsami.3c01454 | DOI Listing |
J Hazard Mater
January 2025
Jiangsu Key Laboratory of Advanced Metallic Materials, School of Materials Science and Engineering, Southeast University, Southeast Road 2nd, Nanjing 211189, PR China. Electronic address:
Oil-in-water (O/W) nanoemulsions, prevalent in the cosmetics, pharmaceutical, and petroleum industries, present significant threats to aquatic ecosystems and human health upon their inadvertent release into the environment. However, the nanoscale droplet size and robust interfacial film of nanoemulsions confer exceptional stability, rendering their separation a formidable challenge. Developing an economical and efficient method to remove nanoemulsions is crucial, offering a cost-effective and energy-saving alternative to traditional techniques.
View Article and Find Full Text PDFSmall
October 2024
State Key Laboratory of Robotics and Systems, School of Mechatronics Engineering, Harbin Institute of Technology, Harbin, 150001, China.
Sweat passive-cooling textiles with asymmetric wettabilities on different sides offer an effective and low-energy consumption solution to personal thermal management in extreme thermal environments. However, the sweat-wicking and the cooling abilities decrease when the textile is contaminated by low-surface tension oily liquid fouling. The integration of anti-oily liquid fouling and sweat-wicking abilities on textile involves resolving the contradiction between hydrophilic and oleophobic properties and seeking eco-friendly short-chain fluorides to reduce the surface energy.
View Article and Find Full Text PDFHeliyon
December 2023
Beijing Key Laboratory of Clothing Materials R & D and Assessment, Beijing Engineering Research Center of Textile Nanofiber, School of Materials Design & Engineering, Beijing Institute of Fashion Technology, Beijing, 100029, China.
The rapid development of society and industry as well as the frequent occurrence of oil spills cause the shortage of fresh water resources, which not only affects human safety and life, but also impedes the world-wide sustainable development. To address these challenges, novel membrane materials with unique wettability properties have gained significant attention, particularly in the field of oil/water separation. In this research, we modified the hydrophobic PET fabric to achieve superhydrophilic characteristics using impregnation method.
View Article and Find Full Text PDFACS Appl Mater Interfaces
May 2023
Key Laboratory of Bio-inspired Smart Interfacial Science and Technology, School of Chemistry, Beihang University, Beijing 102206, P. R. China.
Unidirectional and long-distance liquid transport is critically important to a range of practical applications, e.g., water harvesting, microfluidics, and chemical reactions.
View Article and Find Full Text PDFSci Adv
July 2020
Department of Mechanical Engineering, City University of Hong Kong, Hong Kong, P. R. China.
Despite their simplicity, water droplets manifest a wide spectrum of forms and dynamics, which can be actuated using special texture at solid surfaces to achieve desired functions. Along this vein, natural or synthetic materials can be rendered water repellent, oleophobic, antifogging, anisotropic, etc.-all properties arising from an original design of the substrate and/or from the use of special materials promoting capillary or elastic forces at the droplet scale.
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