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The dynamics of levitated liquid droplets can be used to measure their thermophysical properties by correlating the frequencies at which normal modes of oscillation most strongly resonate when subject to an external oscillatory force. In two preliminary works, it was shown via electrostatic levitation and processing of various metals and alloys that (1) the resonance of the first principal mode of oscillation (mode n = 2) can be used to accurately measure surface tension and (2) that so-called "higher-order resonance" of n = 3 is observable at a predictable frequency. It was also shown, in the context of future space-based experimentation on the Electrostatic Levitation Furnace (ELF), a setup on the International Space Station (ISS) operated by Japan Aerospace Exploration Agency (JAXA), that while the shadow array method in which droplet behavior is visualized would be challenging to identify the n = 3 resonance, the normal mode n = 4 was predicted to be more easily identifiable. In this short communication, experimental evidence of the first three principal modes of oscillation is provided using molten samples of Tin and Indium and it is subsequently shown that, as predicted, an "image-less" approach can be used to identify both n = 2 and n = 4 resonances in levitated liquid droplets. This suggests that the shadow array method may be satisfactorily used to obtain a self-consistent benchmark of thermophysical properties by comparing results from two successive even-mode natural frequencies.
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http://dx.doi.org/10.1038/s41526-023-00254-7 | DOI Listing |
Langmuir
September 2025
School of Energy and Power Engineering, Shandong University, Jinan 250061, China.
Recent advances in microfluidic technology have positioned droplet-based systems as versatile microreactors, leveraging their unique interfacial dynamics and mass transfer properties. While precise manipulation of gas-liquid interfaces or external fields enables controlled chemical reactions and drug synthesis, escalating system complexity demands enhanced regulation of droplet thermodynamics and kinetics. The Leidenfrost phenomenon demonstrates significant engineering potential through its capacity to spontaneously form vapor lubrication layers, facilitating noncontact suspension and controlled evaporation of droplets.
View Article and Find Full Text PDFNPJ Microgravity
August 2025
Institute of Space and Astronautical Science, Japan Aerospace Exploration Agency, 2-1-1 Sengen, Tsukuba, Ibaraki, 305-8505, Japan.
The LaO-NbO binary system is a unique glass-forming system without conventional network former oxides, exhibiting two distinct glass-forming regions: LaO-rich and NbO-rich compositions. To evaluate its glass-forming ability, the temperature dependence of density, viscosity, and surface tension was measured using the electrostatic levitation furnace aboard the International Space Station (ISS-ELF). Melt density showed linear temperature dependence, and thermal expansion coefficients at 2000 K varied from 2.
View Article and Find Full Text PDFJ Environ Sci (China)
December 2025
Department of Chemistry and Chemical Engineering, Chalmers University of Technology, Gothenburg 41296, Sweden. Electronic address:
Alkanes are present in the atmosphere, commonly in the form of aerosols, and can thus interact with water droplets, leading to the formation of new interfaces. Yet, in the study of these interactions, traditional experimental methods often rely on the presence of sample containers, which can interfere with the observations. Acoustic levitation is a technique which allows the manipulation of samples in the microliter regime in a contact-free manner.
View Article and Find Full Text PDFACS Omega
July 2025
Key Laboratory of Mechanics, Anhui Polytechnic University, Wuhu, Anhui 241000, China.
In this paper, we numerically investigate the levitation behaviors of a drop impacting an immiscible liquid-liquid interface, disregarding the influence of gravitational acceleration. Through energy budget analysis, we elucidate that the phenomenological model proposed by Sanjay et al. (, vol.
View Article and Find Full Text PDFPhys Chem Chem Phys
August 2025
Chemical Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, CA 94720, USA.
Microdroplets are purported to enhance reaction rates and produce spontaneous chemical transformations that are unfavorable in macroscale systems. The gas-liquid interface is widely implicated for the emergence of these chemical anomalies. Experiments conducted on individual microdroplets provide a unique platform for studying interfacial effects while bypassing transport limitations often encountered in macroscopic systems.
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