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Characterizing the properties of X-ray free-electron laser (XFEL) sources is a critical step for optimization of performance and experiment planning. The recent availability of MHz XFELs has opened up a range of new opportunities for novel experiments but also highlighted the need for systematic measurements of the source properties. Here, MHz-enabled beam imaging diagnostics developed for the SPB/SFX instrument at the European XFEL are exploited to measure the shot-to-shot intensity statistics of X-ray pulses. The ability to record pulse-integrated two-dimensional transverse intensity measurements at multiple planes along an XFEL beamline at MHz rates yields an improved understanding of the shot-to-shot photon beam intensity variations. These variations can play a critical role, for example, in determining the outcome of single-particle imaging experiments and other experiments that are sensitive to the transverse profile of the incident beam. It is observed that shot-to-shot variations in the statistical properties of a recorded ensemble of radiant intensity distributions are sensitive to changes in electron beam current density. These changes typically occur during pulse-distribution to the instrument and are currently not accounted for by the existing suite of imaging diagnostics. Modulations of the electron beam orbit in the accelerator are observed to induce a time-dependence in the statistics of individual pulses - this is demonstrated by applying radio-frequency trajectory tilts to electron bunch-trains delivered to the instrument. We discuss how these modifications of the beam trajectory might be used to modify the statistical properties of the source and potential future applications.
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http://dx.doi.org/10.1107/S1600577522005720 | DOI Listing |
J Phys Chem Lett
September 2025
Sorbonne Université, CNRS, UMR 7614, Laboratoire de Chimie Physique-Matière et Rayonnement, F-75005 Paris, France.
We report carbon and fluorine KV double core hole (DCH) spectra of CHF, recorded by single-photon hard X-ray photoelectron spectroscopy. A striking inversion in intensity between the and K7(3) resonances reflects a polarity switch in bonding character depending on the K-shell vacancy site. Within the Brillouin Inverse Theorem (BIT) framework, the transition strengths are shown to depend on the bielectronic integral (V = σ*, 3).
View Article and Find Full Text PDFNat Commun
August 2025
European XFEL, Schenefeld, Germany.
A fundamental understanding of the interplay between lattice structure, polarization and electrons is pivotal to the optical control of ferroelectrics. The interaction between light and matter enables the remote and wireless control of the ferroelectric polarization on the picosecond timescale, while inducing strain, i.e.
View Article and Find Full Text PDFJ Synchrotron Radiat
September 2025
Department of Clinical Medicine, Aarhus University, Aarhus, Denmark.
Characterization of the stray radiation field present in the undulator systems at the European XFEL GmbH (EuXFEL) is of great importance, as the potential damage to undulator permanent magnets, electronics and diagnostic equipment depends both on the type of particles and the energy. This work presents the energy profile of the stray radiation measured in the upstream and downstream part of the undulator system near the beam pipe. The influence of machine operation settings on the radiation field intensity was also investigated.
View Article and Find Full Text PDFNPJ Comput Mater
August 2025
Laboratory for Solid State Physics, ETH Zurich, Zürich, Switzerland.
Coherent Diffraction Imaging (CDI) is an experimental technique to image isolated structures by recording the scattered light. The sample density can be recovered from the scattered field through a Fourier Transform operation. However, the phase of the field is lost during the measurement and has to be algorithmically retrieved.
View Article and Find Full Text PDFJ Synchrotron Radiat
September 2025
ESRF - The European Synchrotron, 71 avenue des Martyrs, 38000 Grenoble, France.
The fastest pixel array X-ray detectors can record images with nanosecond resolution. This is accomplished by storing only a few images in in-pixel memory cells. In this study, we demonstrate nanosecond resolution over a large number of images by operating a prototype detector in an event driven mode.
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