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Electron correlation and topology are two central threads of modern condensed matter physics. Semiconductor moiré materials provide a highly tuneable platform for studies of electron correlation. Correlation-driven phenomena, including the Mott insulator, generalized Wigner crystals, stripe phases and continuous Mott transition, have been demonstrated. However, non-trivial band topology has remained unclear. Here we report the observation of a quantum anomalous Hall effect in AB-stacked MoTe /WSe moiré heterobilayers. Unlike in the AA-stacked heterobilayers, an out-of-plane electric field not only controls the bandwidth but also the band topology by intertwining moiré bands centred at different layers. At half band filling, corresponding to one particle per moiré unit cell, we observe quantized Hall resistance, h/e (with h and e denoting the Planck's constant and electron charge, respectively), and vanishing longitudinal resistance at zero magnetic field. The electric-field-induced topological phase transition from a Mott insulator to a quantum anomalous Hall insulator precedes an insulator-to-metal transition. Contrary to most known topological phase transitions, it is not accompanied by a bulk charge gap closure. Our study paves the way for discovery of emergent phenomena arising from the combined influence of strong correlation and topology in semiconductor moiré materials.
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http://dx.doi.org/10.1038/s41586-021-04171-1 | DOI Listing |
Nanoscale
September 2025
St. Petersburg State University, 199034 St. Petersburg, Russia.
Using angle-resolved photoemission spectroscopy (ARPES) with spin resolution, scanning tunneling microscopy/spectroscopy (STM/STS) and density functional theory (DFT) methods, we study the electronic structure of graphene-covered and bare Au/Co(0001) systems and reveal intriguing features, arising from the ferrimagnetic order in graphene and the underlying gold monolayer. In particular, a spin-polarized Dirac-cone-like state, intrinsically related to the induced magnetization of Au, was discovered at point. We have obtained a good agreement between experiment and theory for bare and graphene-covered Au/Co(0001) and have proven that both Au ferrimagnetism and the Dirac-cone-like band are intimately linked to the triangular loop dislocations present at the Au/Co interface.
View Article and Find Full Text PDFACS Nano
September 2025
Hefei National Research Center for Physical Sciences at the Microscale, CAS Key Laboratory of Strongly-Coupled Quantum Matter Physics, Department of Physics, University of Science and Technology of China, Hefei, Anhui 230026, China.
As a versatile platform for exploring exotic quantum phases, moiré superlattices, ranging from twisted graphene to twisted transition metal dichalcogenides, have been intensively studied. In this work, based on exact diagonalization and Hartree-Fock mean-field calculations, the interaction-driven topological phases are investigated in hole-doped twisted bilayer MoS at the high filling factor = 3. Besides the nematic insulator and quantum anomalous Hall phases, the topological Wigner molecule crystal (TWMC) phase is found in the phase diagram.
View Article and Find Full Text PDFACS Nano
September 2025
Ultrafast Electron Microscopy Laboratory, The MOE Key Laboratory of Weak-Light Nonlinear Photonics, School of Physics, Nankai University, Tianjin 300071, China.
Superlattices (SLs) based on two-dimensional (2D) van der Waals (vdW) materials, abbreviated as 2D-SLs, have garnered significant attention due to their customizable properties. 2D-SLs can be engineered by mechanical stacking or chemical intercalation to achieve diverse forms of symmetry breaking, resulting in exotic phenomena like the quantum anomalous Hall effect and topological magnetism. Hitherto, broken symmetries in 2D-SLs have been widely produced within lateral planes or three dimensions.
View Article and Find Full Text PDFJ Phys Chem Lett
September 2025
School of Physics and Beijing Key Laboratory of Optoelectronic Functional Materials & MicroNano Devices, Renmin University of China, Beijing 100872, China.
The interplay between topology and magnetism induces various exotic quantum phenomena, with magnetic topological insulators (MTIs) serving as a prominent example due to their ability to host the quantum anomalous Hall effect (QAHE). However, the realization of the QAHE at a higher temperature approaching the magnetic transition temperature remains a significant challenge, primarily due to the scarcity of suitable material platforms and our limited understanding of the intricate relationships among band topology, magnetism, and defects. Here, we report a comprehensive investigation of MnSbTe·(SbTe) ( = 0-5) single crystals, including the discovery of the novel MnSbTe pure phase.
View Article and Find Full Text PDFAdv Mater
September 2025
School of Physics and Astronomy, Tel Aviv University, Tel Aviv, 6997801, Israel.
Graphene layers can assemble in two shifted metastable positions per interface, leading to eight possible structural arrangements in five-layer graphene, six of which correspond to distinct periodic crystals. These polytypes exhibit diverse symmetries, interlayer electronic hybridization, van der Waals adhesion, and optical responses. Arrangements lacking inversion [I] and mirror [M] symmetries host intrinsic polarizations, while those with sufficiently flat electronic bands display orbital magnetization, unconventional superconductivity, and anomalous fractional quantum Hall states.
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