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High T_{c} superconductors show a rich variety of phases associated with their charge degrees of freedom. Valence charges can give rise to charge ordering or acoustic plasmons in these layered cuprate superconductors. While charge ordering has been observed for both hole- and electron-doped cuprates, acoustic plasmons have only been found in electron-doped materials. Here, we use resonant inelastic x-ray scattering to observe the presence of acoustic plasmons in two families of hole-doped cuprate superconductors (La_{1.84}Sr_{0.16}CuO_{4} and Bi_{2}Sr_{1.6}La_{0.4}CuO_{6+δ}), crucially completing the picture. Interestingly, in contrast to the quasistatic charge ordering which manifests at both Cu and O sites, the observed acoustic plasmons are predominantly associated with the O sites, revealing a unique dichotomy in the behavior of valence charges in hole-doped cuprates.
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http://dx.doi.org/10.1103/PhysRevLett.125.257002 | DOI Listing |
RSC Chem Biol
August 2025
Department of Chemistry - BMC, Uppsala University Sweden
Analysis of ligand-induced structural changes in proteins is challenging due to the lack of experimental methods suited for detection and characterisation of both ligand binding and induced structural changes. We have explored biosensors with different detection principles to study interactions between ligands and acetylcholine binding proteins (AChBPs), soluble homologues of Cys-loop ligand gated ion channels (LGICs) that undergo similar structural changes as LGICs upon ligand binding. X-ray crystallography was used to identify binding sites and establish if the detected conformational changes involved small changes in loop C or major structural changes in the pentamer associated with ion channel opening.
View Article and Find Full Text PDFNano Lett
August 2025
Faculty of Physics and Astronomy, Adam Mickiewicz University, Uniwersytetu Poznanskiego 2, Poznan 61-614, Poland.
Nanocomposites assembled from polymer-grafted plasmonic nanoparticles (PGNs) can combine strong light-matter interactions with soft-matter functionalities and a high degree of translational symmetry. This work explored the potential of gold nanoparticles (16 nm diameter) grafted with polystyrene chains (degree of polymerization, ≈ 63) as building blocks for acoustoplasmonic metasurfaces. We have decorated inorganic surfaces─crystalline silicon and SiO glass─with PGN monolayers and explored their surface acoustic waves with micro-Brillouin Light Scattering (μ-BLS) at various photon energies.
View Article and Find Full Text PDFScience
July 2025
Geballe Laboratory for Advanced Materials, Stanford University, Stanford, CA, USA.
The important role of metallic nanostructures in nanophotonics will expand if ways to electrically manipulate their optical resonances at high speed can be identified. We capitalized on electrically driven surface acoustic waves and the extreme light concentration afforded by gap plasmons to achieve this goal. We placed gold nanoparticles in a particle-on-mirror configuration with a few-nanometer-thick, compressible polymer spacer.
View Article and Find Full Text PDFEnhancing light-matter interaction through deep subwavelength-scale confinement is crucial for numerous applications like molecular sensing, optoelectronic devices, and non-linear optics. Here, we report the excitation of localized acoustic graphene plasmons (LAGPs) confined in a sub-micro- wide, nanometer-thick layer using a metal slit antenna. This approach enables light funneling in the infrared and terahertz regimes, leading to strong field enhancement and confinement.
View Article and Find Full Text PDFACS Appl Mater Interfaces
June 2025
State Key Laboratory of Electronic Thin Film and Integrated Devices, University of Electronic Science and Technology of China, Chengdu 610054, China.
High-responsivity and broad-spectrum photodetectors are indispensable for advanced photoelectric applications. While silicon PIN junctions offer several advantages, such as mature manufacturing processes, stable performance, and cost-effectiveness, their near-infrared detection capabilities are fundamentally constrained by the intrinsic properties of silicon. In this study, we propose a device structure that advances photodetection beyond the limitation of silicon PIN junctions by in situ integrating randomly interlinked gold nanoparticles and black silicon (RIL-AuNPs/B-Si).
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