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Spatial catalytic acid-base-Pd triple-sites of a hierarchical core-shell structure have been successfully constructed for a three-step reaction, and exhibited excellent catalytic activity and stability. A catalytic mechanism has been systematically studied via single one- and two-step reactions, and possible molecular reactions have been proposed.
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http://dx.doi.org/10.1039/d0cc01701a | DOI Listing |
Chem Commun (Camb)
June 2020
School of Chemistry, Chemical Engineering and Life Science and State Key Laboratory of Advanced Technology for Materials Synthesis and Processing, Materials Science & Engineering, Wuhan University of Technology, 122, Luoshi Road, 430070, Wuhan, Hubei, China.
Spatial catalytic acid-base-Pd triple-sites of a hierarchical core-shell structure have been successfully constructed for a three-step reaction, and exhibited excellent catalytic activity and stability. A catalytic mechanism has been systematically studied via single one- and two-step reactions, and possible molecular reactions have been proposed.
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