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We present the results of a muon spin relaxation study of the solid phases of the expanded metal, Li(NH3)4. No discernible change in muon depolarization dynamics is witnessed in the lowest temperature phase (≤25 K) of Li(NH3)4, thus suggesting that the prevailing view of antiferromagnetic ordering is incorrect. This is consistent with the most recent neutron diffraction data. Discernible differences in muon behavior are reported for the highest temperature phase of Li(NH3)4 (82-89 K), attributed to the onset of structural dynamics prior to melting.
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http://dx.doi.org/10.1021/acs.jpclett.5b01380 | DOI Listing |
Adv Mater
September 2025
Dept. of Physics, Pennsylvania State University, University Park, PA, 16802, USA.
Altermagnets are a newly identified family of collinear antiferromagnets with a momentum-dependent spin-split band structure of non-relativistic origin, derived from spin-group symmetry-protected crystal structures. Among candidate altermagnets, CrSb is attractive for potential applications because of a large spin-splitting near the Fermi level and a high Néel transition temperature of around 700 K. Molecular beam epitaxy is used to synthesize CrSb (0001) thin films with thicknesses ranging from 10 to 100 nm.
View Article and Find Full Text PDFJ Am Chem Soc
September 2025
Institute of Inorganic and Analytical Chemistry, University of Münster, Corrensstrasse 28/30, 48149 Münster, Germany.
Materials exhibiting coexisting exploitable properties often result in especially attractive behavior from both fundamental and applied perspectives. In particular, magnetoelectric materials combining ferroelectric and magnetic properties are increasingly becoming paramount nowadays. Here, we show that FeH(PO) exhibits proton conductivity and the coexistence of magnetic and polar structural features, suggesting that such frameworks may be of broader interest beyond the field of proton conductors.
View Article and Find Full Text PDFSmall
September 2025
Department of Materials Science, Chiba University, 1-33 Yayoi-cho, Inage-ku, Chiba, 263-8522, Japan.
1D electronic structures on 2D crystalline surfaces are crucial for investigating low-dimensional quantum phenomena and enabling the development of dimensionally engineered nanodevices. However, the inherent periodic symmetry of 2D atomic lattices generally leads to delocalized electronic band extending across the surface, making the creation of periodic 1D electronic states a significant challenge. Here, robust 1D electronic ordering is demonstrated in ultrathin Mn films grown on an atomically flat, non-reconstructed body-centered cubic Fe substrate.
View Article and Find Full Text PDFACS Nano
September 2025
Instituto de Ciencia de Materiales de Barcelona. ICMAB-CSIC. Campus Universitario UAB, Bellaterra 08193, Spain.
In this work, we investigate how the crystallographic growth direction influences spin current transmission in antiferromagnetic (AF) NiO thin films. By manipulating epitaxial growth, we explored the spin transport characteristics in LaSrMnO/NiO/Pt heterostructures grown on top of (001)- and (111)-oriented SrTiO substrates, varying the NiO barrier thickness (t). Spin currents were generated via spin pumping (SP), and detection was done by the inverse spin Hall effect (ISHE).
View Article and Find Full Text PDFRep Prog Phys
September 2025
TU Dresden, Institut für Theoretische Physik, Dresden, 01062, GERMANY.
A central concept in the theory of phase transitions beyond the Landau-Ginzburg-Wilson paradigm is fractionalization: the formation of new quasiparticles that interact via emergent gauge fields. This concept has been extensively explored in the context of continuous quantum phase transitions between distinct orders that break different symmetries. We propose a mechanism for continuous order-to-order quantum phase transitions that operates independently of fractionalization.
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