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We theoretically analyze plasmonic gap-mode nanocavities covered by a thick cladding layer at telecommunication wavelengths. In the presence of high-index cladding materials such as semiconductors, the first-order hybrid gap mode becomes more promising for lasing than the fundamental one. Still, the significant mirror loss remains the main challenge to lasing. Using silver coatings within a decent thickness range at two end facets, we show that the reflectivity is substantially enhanced above 95 %. At a coating thickness of 50 nm and cavity length of 1.51 μm, the quality factor is about 150, and the threshold gain is lower than 1500 cm(-1).
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http://dx.doi.org/10.1364/OE.21.013479 | DOI Listing |
In applications such as plasmonic sensors and plasmonic nanolasers, constructing metal nanostructures with a wide range of tunability of plasmonic dephasing times is becoming increasingly important. However, the manipulation range of the dephasing time is still limited from only a few femtoseconds to tens of femtoseconds. Here, we propose what we believe to be a novel method to greatly extend the tunable range of plasmonic dephasing time by leveraging the strong coupling between the plasmonic gap mode and the surface lattice resonance mode.
View Article and Find Full Text PDFAnalyst
July 2025
School of Chemistry, University of Nottingham, University Park, Nottingham, NG7 2RD, UK.
Benchmarking the near-field signal enhancement attained using plasmonic metal-coated atomic force microscopy (AFM) probes for tip-enhanced Raman spectroscopy (TERS) and tip-enhanced photoluminescence (TEPL) measurements is challenging given the absence of a suitable reference sample that is simple to prepare, easy to use and compatible with different instrument configurations. To this end, in this study, we have fabricated a flake of monolayer tungsten diselenide (1L-WSe) stamped across the interface of gold and silver thin films on silicon dioxide and glass. We have demonstrated these samples to be effective for the facile determination of near-field Raman and photoluminescence contrast factors in both gap and non-gap mode, respectively.
View Article and Find Full Text PDFNanophotonics
March 2024
Institute of Physical and Theoretical Chemistry, Eberhard Karls University of Tübingen, 72076 Tübingen, Germany.
ACS Appl Mater Interfaces
October 2024
School of Electrical Engineering, Korea Advanced Institute of Science and Technology (KAIST), 291 Daehak-ro, Yuseong-gu, Daejeon 34141, Republic of Korea.
Plasmon resonance using metal nanostructures enables the realization of high-performance optoelectronic devices via field enhancements in the vicinity of the metal nanostructure. This study proposes an ultrabroadband MoS photodetector based on the gap-mode plasmon of gold nanorods. The use of MoS as a gap spacer for the gap-mode plasmon effect and as a channel material for the photodetector is demonstrated.
View Article and Find Full Text PDFNat Commun
May 2024
Department of Physics, Emory University, Atlanta, GA, 30322, USA.
Photoluminescence from spatially inhomogeneous plasmonic nanostructures exhibits fascinating wavelength-dependent nonlinear behaviors due to the intraband recombination of hot electrons excited into the conduction band of the metal. The properties of the excited carrier distribution and the role of localized plasmonic modes are subjects of debate. In this work, we use plasmonic gap-mode resonators with precise nanometer-scale confinement to show that the nonlinear photoluminescence behavior can become dominated by non-thermal contributions produced by the excited carrier population that strongly deviates from the Fermi-Dirac distribution due to the confinement-induced large-momentum free carrier absorption beyond the dipole approximation.
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