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The statistical mechanics of the time-reversal and inversion symmetry breaking order parameter, possibly observed in the pseudogap region of the phase diagram of the cuprates, can be represented by the Ashkin-Teller model. We add kinetic energy and dissipation to the model for a quantum generalization and show that the spectrum of the quantum-critical fluctuations is of the form postulated in 1989 to give the marginal Fermi-liquid properties. The model solved and the methods devised are likely to be of interest also to other quantum phase transitions.
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http://dx.doi.org/10.1103/PhysRevLett.99.067003 | DOI Listing |
J Chem Theory Comput
September 2025
Materials DX Research Center, National Institute of Advanced Industrial Science and Technology, Tsukuba Central 2, 1-1-1 Umezono, Tsukuba, Ibaraki 305-8568, Japan.
The quantum mechanics/molecular mechanics (QM/MM) method is a powerful approach for investigating solid surfaces in contact with various types of media, since it allows for flexible modeling of complex interfaces while maintaining an all-atom representation. The mean-field QM/MM method is an average reaction field model within the QM/MM framework. The method addresses the challenges associated with the statistical sampling of interfacial atomic configurations of a medium and enables efficient calculation of free energies.
View Article and Find Full Text PDFPhys Rev Lett
August 2025
McMaster University, Department of Physics and Astronomy, Hamilton, Ontario L8S 4M1, Canada.
Magnetic heat capacity measurements of a high-quality single crystal of the dipole-octupole pyrochlore Ce_{2}Hf_{2}O_{7} down to a temperature of T=0.02 K are reported. These show a two-peaked structure, with a Schottky-like peak at T_{1}∼0.
View Article and Find Full Text PDFPhys Rev Lett
August 2025
University of Science and Technology of China, Hefei National Research Center for Physical Sciences at the Microscale and Synergetic Innovation Center of Quantum Information & Quantum Physics, New Cornerstone Science Laboratory, Hefei, Anhui 230026, China.
The multiplicity of orbitals in quantum systems significantly influences the competition between Kondo screening and local spin magnetization. The identification of orbital-specific processes is essential for advancing spintronic devices, as well as for enhancing the understanding of many-body quantum phenomena, but it remains a great challenge. Here, we use a combination of scanning tunneling microscopy/spectroscopy and electron spin resonance (ESR) spectroscopy to investigate single iron phthalocyanine (FePc) molecules on MgO/Ag(100).
View Article and Find Full Text PDFACS Nano
September 2025
School of Physics and Key Lab of Quantum Materials and Devices of the Ministry of Education, Southeast University, Nanjing 211189, P. R. China.
While hexagonal boron nitride (hBN) hosts promising room-temperature quantum emitters for hybrid quantum photonic circuits, scalable deterministic integration and insufficient brightness alongside low photon collection and coupling efficiencies remain unresolved challenges. We present a femtosecond laser nanoengineering platform that enables the site-specific generation of hBN single-photon source (SPS) arrays. First-principles density functional theory (DFT) calculations and polarization-resolved spectroscopy confirm the atomic origin of emission as interfacial defects at hBN/SiO heterojunctions.
View Article and Find Full Text PDFPhys Rev Lett
August 2025
ShanghaiTech University, School of Physical Science and Technology, Shanghai 201210, China.
We report direct spectroscopic evidence of correlation-driven Mott states in layered Nb_{3}Cl_{8} through combining scanning tunneling microscopy (STM) and dynamical mean-field theory. The Hubbard bands persist down to monolayer, providing the definitive evidence for the Mottness in Nb_{3}Cl_{8}. While the size of the Mott gap remains almost constant across all layers, a striking layer-parity-dependent oscillation emerges in the local density of states (LDOS) between even (n=2, 4, 6) and odd layers (n=1, 3, 5), which arises from the dimerization and correlation modulation of the obstructed atomic states, respectively.
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