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Electro-optical modulation is essential in optical signal processing and laser technology, yet modulators based on the Pockels effect in flat optics lag behind bulk and integrated platforms in efficiency and speed. We bridge this gap realizing a metasurface based on lithium niobate (LiNbO₃) on insulator that leverages on resonances with quality-factor as high as 8000 to achieve fast electrical modulation of both linear and nonlinear optical properties. LiNbO, well known for its high nonlinear susceptibility and wide transparency window across the infrared and visible spectrum, is employed to realize an asymmetric, one-dimensional array of nanowires, exhibiting resonances with linewidth <0.2 nm. The metasurface achieves a reflectivity modulation around 0.1, with a modulation efficiency, defined as relative modulation per applied Volt, larger than 0.01 V on a -3 dB (-6 dB) bandwidth of about 800 MHz (1.4 GHz). Additionally, we demonstrate more than one order of magnitude intensity modulation of the second harmonic seeded by a continuous-wave laser, with a modulation efficiency of about 0.12 V. This dual modulation capability, rooted in the interplay between optical resonances and electric field manipulation, holds significant potential for cutting-edge applications in high-speed photonics, nonlinear optics, and reconfigurable communication systems.
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http://dx.doi.org/10.1038/s41467-025-62072-7 | DOI Listing |
Nanoscale Horiz
August 2025
Department of Physics, National Taiwan Normal University, Taipei 11677, Taiwan.
Transition metal dichalcogenide (TMD) materials, such as molybdenum disulfide (MoS), have emerged as promising platforms for exploring electrically tunable light-matter interactions, which are critical for designing high-performance photodetector systems. In this study, we investigate the advancements in quantum tunneling MoS field-effect transistors (QT-MoS FETs) and their optoelectronic properties, with a focus on photoresponse behavior and photoluminescence (PL) spectral variations driven by photoinduced tunneling currents through oxide layers. The results demonstrate that tunneling-induced exciton and trion dissociation effects lead to a pronounced blue shift in PL spectral peaks and significant changes in light intensity.
View Article and Find Full Text PDFACS Photonics
August 2025
Department of Physics, University of Washington, Seattle, Washington 98195, United States.
Triggered by advances in atomic-layer exfoliation and growth techniques, along with the identification of a wide range of extraordinary physical properties in self-standing films consisting of one or a few atomic layers, two-dimensional (2D) materials such as graphene, transition metal dichalcogenides (TMDs), and other van der Waals (vdW) crystals now constitute a broad research field expanding in multiple directions through the combination of layer stacking and twisting, nanofabrication, surface-science methods, and integration into nanostructured environments. Photonics encompasses a multidisciplinary subset of those directions, where 2D materials contribute remarkable nonlinearities, long-lived and ultraconfined polaritons, strong excitons, topological and chiral effects, susceptibility to external stimuli, accessibility, robustness, and a completely new range of photonic materials based on layer stacking, gating, and the formation of moiré patterns. These properties are being leveraged to develop applications in electro-optical modulation, light emission and detection, imaging and metasurfaces, integrated optics, sensing, and quantum physics across a broad spectral range extending from the far-infrared to the ultraviolet, as well as enabling hybridization with spin and momentum textures of electronic band structures and magnetic degrees of freedom.
View Article and Find Full Text PDFNanoscale Adv
August 2025
Research Center for Applied Sciences (RCAS), Academia Sinica Taipei 11529 Taiwan
We demonstrate a dual-colored light-emitting device using 2D semiconductors by modulating AC carrier injection through independent electrodes with phase delay, enabling balanced emission from WSe and WS monolayers. This innovative approach allows balanced, dynamically controllable, and spectrally stable emissions from WSe and WS monolayers, significantly enhancing emission control and expanding possibilities in advanced multicolor optoelectronic applications, including integrated photonic circuits and high-resolution display technologies.
View Article and Find Full Text PDFAcc Chem Res
September 2025
State Key Lab of Supramolecular Structure and Materials, College of Chemistry, Jilin University, Changchun 130012, People's Republic of China.
ConspectusThe rapid evolution of human-machine interaction frameworks and global digitization initiatives has imposed heightened requirements for intelligent display systems. Electrochromic (EC) non-emissive displays, which dynamically modulate optical properties (e.g.
View Article and Find Full Text PDFSmall
August 2025
Institute for Advanced Materials and Technology, University of Science and Technology Beijing, Beijing, 100083, China.
Polymer dispersed liquid crystal (PDLC) exhibits excellent electro-optical properties for displays and smart windows but lacks sufficient near-infrared modulation for full solar management. Herein, a composite film with dual electrical-thermal control is designed for this purpose, which integrates PDLC film as an electrochromic layer and tungsten-doped vanadium dioxide (W/VO) coating as a thermochromic layer. The composite film not only facilitates active regulation of visible light through electrical control, but also enables the modulation of near-infrared light via phase transitions in response to temperature changes.
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