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The poor interfacial adhesion between ductile gold (Au) electrodes and polydimethylsiloxane (PDMS) substrates affects their application in flexible sensors. Here, a porous Au electrode is designed and combined with a flexible PDMS substrate to form a structure that embeds Au into the PDMS film, thereby enhancing the interfacial adhesion of the Au/PDMS electrode. The resistivity change of the Au/PDMS electrode is only 12.3% after 100 tape peeling trials. The resistance of the Au/PDMS electrode remains stable at the 30% strain level after 2000 tensile cycling tests. This feature is mainly attributed to the deformation buffering effect of the porous Au film. After 100 min of ultrasonic oscillation testing, the resistivity change of the Au/PDMS electrode remains stable. It is also shown that the Au/PDMS electrode has excellent interfacial adhesion properties, which is mainly attributed to the interlocking effect of the Au/PDMS electrode structure. In addition, the temperature coefficient of resistance (TCR) of the temperature sensor based on the Au/PDMS electrode is approximately 0.00320/°C and the sensor's sensitivity remains almost stable after 200 temperature measurement cycles. Au/PDMS electrodes have great potential for a wide range of applications in flexible electronics due to their excellent interfacial adhesion and electrical stability.
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http://dx.doi.org/10.3390/nano15131001 | DOI Listing |
Nanomaterials (Basel)
June 2025
School of Power and Electrical Engineering, Luoyang Institute of Science and Technology, Luoyang 471023, China.
The poor interfacial adhesion between ductile gold (Au) electrodes and polydimethylsiloxane (PDMS) substrates affects their application in flexible sensors. Here, a porous Au electrode is designed and combined with a flexible PDMS substrate to form a structure that embeds Au into the PDMS film, thereby enhancing the interfacial adhesion of the Au/PDMS electrode. The resistivity change of the Au/PDMS electrode is only 12.
View Article and Find Full Text PDFNano Lett
March 2025
Leibniz-Institut für Polymerforschung Dresden e.V, Hohe Straße 6, 01069 Dresden, Germany.
Wireless strain sensors with minimal power needs are essential for long-term monitoring in energy-limited environments. We present a soft tunneling barrier-integrated gold thin film for negative strain sensing with near-zero energy consumption. The device features a strain-induced transition from an insulating to a metallic state, increasing conductivity by 9 orders of magnitude under a controlled strain.
View Article and Find Full Text PDFAnalyst
March 2022
School of Chemistry and Chemical Engineering, Yangzhou University, Yangzhou 225002, P.R. China.
The development of flexible substrate materials and nanomaterials with high electrochemical performance is of great significance for constructing efficient wearable electrochemical sensors for real-time health monitoring. Herein, a wearable electrochemical sweat sensor based on a Ni-Co MOF nanosheet coated Au/polydimethylsiloxane (PDMS) film was prepared for continuous monitoring of the glucose level in sweat with high sensitivity. First, a stretchable Au/PDMS film based three-electrode system was prepared by chemical deposition of a gold layer on the hydrophilic treated PDMS.
View Article and Find Full Text PDFAdv Mater
June 2020
Innovative Centre for Flexible Devices (iFLEX), Max Planck - NTU Joint Lab for Artificial Senses, School of Materials Science and Engineering, Nanyang Technological University, 50 Nanyang Avenue, Singapore, 639798, Singapore.
On-skin flexible devices provide a noninvasive approach for continuous and real-time acquisition of biological signals from the skin, which is essential for future chronic disease diagnosis and smart health monitoring. Great progress has been achieved in flexible devices to resolve the mechanical mismatching between conventional rigid devices and human skin. However, common materials used for flexible devices including silicon-based elastomers and various metals exhibit no resistance to epidermal surface lipids (skin oil and grease), which restricts the long-term and household usability.
View Article and Find Full Text PDFACS Appl Mater Interfaces
February 2018
National Nanotechnology Center (NANOTEC), NSTDA , 111 Thailand Science Park, Paholyothin Road, KlongLuang, Pathum Thani 12120, Thailand.