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Article Abstract

Studies relied on atmospheric PM data to estimate health risks and sources, but its representativeness for indoor air remains unclear. This study placed an atmospheric PM sampler on the rooftop of a three-story building, and indoor and outdoor (balcony) samples were collected from study houses within a 5 km radius of the atmospheric sampling site during low and high PM seasons to evaluate the representativeness of atmospheric PM data. The average PM concentrations were 15.4 ± 7.1 μg/m (indoor), 18.9 ± 7.0 μg/m (outdoor), and 13.9 ± 6.1 μg/m (atmospheric). Atmospheric PM concentrations were significantly associated with indoor and outdoor PM, but outdoor PM concentrations were higher. Source identification revealed that traffic-related emission was a major contributor to PM across all sites and seasons, while long-range transport from China was another source during the high PM season based on lead isotope ratios. Crustal elements and construction dust, identified through positive matrix factorization, were higher in both indoor and outdoor air than in the atmosphere. Elements from industrial or traffic emissions showed similar concentrations across different sampling sites. The average ratios of indoor to outdoor or atmospheric PM concentrations were 0.84 ± 0.27 and 1.18 ± 0.37, respectively. In conclusion, atmospheric PM can be used to estimate PM exposure and element concentrations from industrial or traffic emissions in indoors; however, it underestimates the contributions of crustal elements and construction dust. Ambient PM samples from outdoor or atmospheric environments should be considered when comparing their influence on indoor air across studies.

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http://dx.doi.org/10.1016/j.envpol.2025.126350DOI Listing

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