Category Ranking

98%

Total Visits

921

Avg Visit Duration

2 minutes

Citations

20

Article Abstract

The significant discrepancy observed between the predicted and experimental switching fields in correlated insulators under a DC electric field far-from-equilibrium necessitates a reevaluation of current microscopic understanding. Here we show that an electron avalanche can occur in the bulk limit of such insulators at arbitrarily small electric field by introducing a generic model of electrons coupled to an inelastic medium of phonons. The quantum avalanche arises by the generation of a ladder of in-gap states, created by a multi-phonon emission process. Hot-phonons in the avalanche trigger a premature and partial collapse of the correlated gap. The phonon spectrum dictates the existence of two-stage versus single-stage switching events which we associate with charge-density-wave and Mott resistive phase transitions, respectively. The behavior of electron and phonon temperatures, as well as the temperature dependence of the threshold fields, demonstrates how a crossover between the thermal and quantum switching scenarios emerges within a unified framework of the quantum avalanche.

Download full-text PDF

Source
http://www.ncbi.nlm.nih.gov/pmc/articles/PMC10203265PMC
http://dx.doi.org/10.1038/s41467-023-38557-8DOI Listing

Publication Analysis

Top Keywords

quantum avalanche
12
electric field
8
avalanche
5
correlated insulator
4
insulator collapse
4
quantum
4
collapse quantum
4
avalanche in-gap
4
in-gap ladder
4
ladder states
4

Similar Publications

Singlet-oxygen, the first excited state of molecular oxygen (O), is a reactive oxygen species that plays a key role as a cytotoxic agent in photodynamic therapy (PDT). In this work, we report a highly light-sensitive detection system based on a single-photon avalanche diode (SPAD) detector and time-correlated single-photon counting (TCPSC) for real-time detection of luminescence signatures from photosensitized singlet-oxygen. Dynamics of singlet-oxygen produced by the excitation of small-scale organic nitrobenzoselenadiazole photosensitizers were extracted with acquisition times as short as 1 second.

View Article and Find Full Text PDF

We present a single-photon-sensitive spectrometer based on a linear array of 512 single-photon avalanche diode detectors with 0.04 nm spectral and 40 ps temporal resolutions. We employ a fast data-driven operation that allows direct measurement of time and frequency for simultaneous single photons, time- and frequency-stamping each single-photon detection.

View Article and Find Full Text PDF

The afterpulse effect is an undesirable phenomenon that occurs in single-photon avalanche diodes (SPADs). SPADs are widely employed in quantum key distribution (QKD) systems. As QKD systems advance to support higher data rates, the minimization of afterpulses becomes increasingly critical.

View Article and Find Full Text PDF

We develop a symmetry-based variational theory that shows the coarse-grained balance of work inflow to heat outflow in a driven, dissipative system relaxed to the golden ratio. Two order-2 Möbius transformations-a self-dual flip and a self-similar shift-generate a discrete non-abelian subgroup of PGL(2,Q(5)). Requiring any smooth, strictly convex Lyapunov functional to be invariant under both maps enforces a single non-equilibrium fixed point: the golden mean.

View Article and Find Full Text PDF

Time-resolved Raman spectroscopy using a CMOS SPAD array to remove fluorescent and fibre Raman backgrounds.

Biomed Opt Express

July 2025

Scottish Universities Physics Alliance (SUPA), Institute of Photonics and Quantum Sciences, Heriot-Watt University, Edinburgh, UK.

Raman spectroscopy is limited by weak signals, fluorescence interference, and fibre-induced backgrounds. To address this, a 512-pixel complementary-metal-oxide semiconductor (CMOS) single-photon avalanche diode (SPAD) line sensor array with on-chip timing electronics was employed to enable the detection of weak Raman signals and use time gating to suppress background fluorescence and fibre-induced Raman signal. The functionality of this compact optical system is initially demonstrated in a free space setup, achieving an improved signal enhancement within shorter measurement times of 30 s.

View Article and Find Full Text PDF