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Article Abstract
Planar carbazole based hexaphyrin-like macrocycles with bis-coordinating cores and box-shaped cyclic BODIPYs were synthesized. Solution and solid-state structure analysis of the free macrocycles indicates an inversion of two pyrrole rings, resulting in a two-dipyrrin-like environment. The BF complexes show large Stokes shifts and exhibit excitonic coupling, fine-tuned by the -substituents.
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Planar hexaphyrin-like macrocycles turning into bis-BODIPYs with box-shaped structures exhibiting excitonic coupling.
Chem Commun (Camb)
November 2021
School of Chemistry, Indian Institute of Science Education and Research Thiruvananthapuram-695551, Maruthamala P.O., Vithura, Kerala, India.
Planar carbazole based hexaphyrin-like macrocycles with bis-coordinating cores and box-shaped cyclic BODIPYs were synthesized. Solution and solid-state structure analysis of the free macrocycles indicates an inversion of two pyrrole rings, resulting in a two-dipyrrin-like environment. The BF complexes show large Stokes shifts and exhibit excitonic coupling, fine-tuned by the -substituents.
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