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The calculations presented here reveal that an electron probe carrying orbital angular momentum is just a particular case of a wider class of electron beams that can be used to measure electron magnetic circular dichroism (EMCD) with atomic resolution. It is possible to obtain an EMCD signal with atomic resolution by simply breaking the symmetry of the electron probe phase distribution using the aberration-corrected optics of a scanning transmission electron microscope. The required phase distribution of the probe depends on the magnetic symmetry and crystal structure of the sample. The calculations indicate that EMCD signals utilizing the phase of the electron probe are as strong as those obtained by nanodiffraction methods.
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http://dx.doi.org/10.1103/PhysRevLett.113.145501 | DOI Listing |
Phys Rev Lett
August 2025
RIKEN Center for Quantum Computing, 2-1 Hirosawa, Wako, Saitama 351-0198, Japan.
We present a method for probing the quantum capacitance associated with the Rydberg transition of surface electrons on liquid helium using radio-frequency (rf) reflectometry. Resonant microwave excitation of the Rydberg transition induces a redistribution of image charges on capacitively coupled electrodes, giving rise to a quantum capacitance originating from adiabatic state transitions and the finite curvature of the energy bands. By applying frequency-modulated resonant microwaves to drive the Rydberg transition, we systematically measured a capacitance sensitivity of 0.
View Article and Find Full Text PDFPhys Rev Lett
August 2025
Huazhong University of Science and Technology, Wuhan National Laboratory for Optoelectronics and School of Physics, Wuhan 430074, China.
We propose a scheme for retrieving the ultrafast valley polarization (VP) dynamics in two-dimensional hexagonal materials via attosecond circular dichroism (CD) transient absorption spectroscopy. This approach builds on the CD transition between the first and higher conduction bands induced by the circularly polarized probe pulses. The population imbalance at nonequivalent valleys in the first conduction band is proportionally mapped onto the difference in absorption coefficients of two probe pulses with opposite helicities, supporting an unprecedented quantitative retrieval of the corresponding VP dynamics with subfemtosecond time resolution.
View Article and Find Full Text PDFJ Phys Chem A
September 2025
Department of Chemistry, Brown University, Providence, Rhode Island 02912, United States.
Chlorothiophenols are key precursors for polychlorinated dibenzothiophenes, which are a class of persistent organic pollutants environmentally, but little is known about their electronic and spectroscopic properties. We report a high-resolution spectroscopic investigation of the cryogenically cooled 2-chlorothiophenoxide (2-CTP) anion using photoelectron imaging, photodetachment spectroscopy, and resonant photoelectron spectroscopy. High-resolution photoelectron spectroscopy yields an accurate electron affinity of 21,005 ± 5 cm (2.
View Article and Find Full Text PDFPhys Rev Lett
August 2025
Sorbonne Université, Laboratoire de physique nucléaire et des hautes énergies (LPNHE), Université Paris Cité, CNRS/IN2P3, Paris, France.
We report on a search for sub-GeV dark matter (DM) particles interacting with electrons using the DAMIC-M prototype detector at the Modane Underground Laboratory. The data feature a significantly lower detector single e^{-} rate (factor 50) compared to our previous search, while also accumulating a 10 times larger exposure of ∼1.3 kg-day.
View Article and Find Full Text PDFPhys Rev Lett
August 2025
Duke University, Thomas Lord Department of Mechanical Engineering and Materials Science, Durham, North Carolina 27708, USA.
Chiral phonons, which are characterized by rotational atomic motion, offer a unique mechanism for transferring angular momentum from phonons to electron spins and other angular momentum carriers. In this Letter, we present a theoretical investigation into the emergence of chiral phonons in a chiral hybrid organic-inorganic perovskite (HOIP) and their critical roles in rigid-body rotation, magnetic moment generation, and spin transport under nonthermal equilibrium conditions. We demonstrate that phonon angular momentum can modify the spin chemical potential via a proposed microscopic Barnett effect, leading to a spatially varying spin chemical potential at the metal/HOIP interface, which subsequently induces spin currents in an adjacent Cu layer, with a magnitude consistent with experimental observations.
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