Publications by authors named "Hyeong Chan Suh"

Correction for 'Mitigating substrate effects of van der Waals semiconductors using perfluoropolyether self-assembled monolayers' by Dae Young Park , , 2024, , 10779-10788, https://doi.org/10.1039/D4NR00061G.

View Article and Find Full Text PDF

Local deformation is a control knob to dynamically tune the electronic band structure of 2D semiconductors. This study demonstrates the local strain-dependent phonon properties of monolayer tungsten diselenide, which are investigated by using the scanning tunneling microscopy-based tip-enhanced Raman spectroscopy. The anomalous appearance and softening of the Raman-inactive out-of-plane mode are first revealed, which exhibits equivalent behavior to other principal phonons of tungsten diselenide.

View Article and Find Full Text PDF

Transition metal dichalcogenide (TMDs) heterostructure, particularly the lateral heterostructure of two different TMDs, is gaining attention as ultrathin photonic devices based on the charge transfer (CT) excitons generated at the junction. However, the characteristics of the interface of the lateral heterostructure, determining the electronic band structure and alignment at the heterojunction region, have rarely been studied due to the limited spatial resolution of nondestructive analysis systems. In this study, we investigated the confined phonons resulting from the phonon-disorder scattering process involving multiple disorders at the lateral heterostructure interface of MoS-WS to prove the consequences of disorder-mediated deformation in the band structure.

View Article and Find Full Text PDF

Brightening dark excitons in transition metal dichalcogenide monolayers (MLs) can provide large-area ultrathin devices for applications in quantum information science and optoelectronics. For practical applications of dark excitons, a robust and bright emission over a wide area at room temperature is desirable; however, no reliable approach has been demonstrated thus far. In this study, an efficient approach is presented for brightening dark excitons at room temperature over a large area of a WSe ML via coupling between plasmons and dark excitons.

View Article and Find Full Text PDF

Recently, 2D semiconductor-based optoelectronic memory has been explored to overcome the limitations of conventional von Neumann architectures by integrating optical sensing and data storage into one device. Persistent photocurrent (PPC), essential for optoelectronic memory, originates from charge carrier trapping according to the Shockley-Read-Hall (SRH) model in 2D semiconductors. The quasi-Fermi level position influences the activation of charge-trapping sites.

View Article and Find Full Text PDF
Article Synopsis
  • The performance of transition metal dichalcogenides (TMDCs) relies heavily on the dielectric constant of the substrates they are placed on, which limits their use in various applications.
  • A solution was developed using a low surface energy perfluorinated polyether (PFPE) self-assembled monolayer (SAM) to increase the distance between TMDCs and their substrates, reducing interactions.
  • This approach led to improved device characteristics, such as lower subthreshold swing, higher photoluminescence intensity of excitons, and reduced substrate doping effects, thereby enhancing the potential applications of TMDCs.
View Article and Find Full Text PDF