Cleaning activities can affect indoor air composition long after the cleaning is completed. Utilizing data from detailed observational monitoring campaigns, conducted over 21 weeks, we explore the influence of cleaning activities in two normally occupied, single-family houses. To study emissions and chemistry, we quantified more than 200 volatile organic compounds (VOCs) using a proton-transfer reaction time-of-flight mass spectrometer and 52 semivolatile organic compounds (SVOCs) using a semivolatile thermal-desorption gas chromatograph.
View Article and Find Full Text PDFEnviron Sci Technol
April 2025
In Los Angeles, air pollution disproportionately impacts communities of color and low-income residents. Routine city-wide measurements of hazardous air pollutants (HAPs), of concern for health and contributing to urban air pollution, are notably lacking. In this study, we use the highest spatially resolved (∼2 km) measurements of emissions and concentrations ever reported of HAPs while covering a whole megacity and combine observations with US Census information.
View Article and Find Full Text PDFEnviron Sci Technol
April 2025
In this study, we evaluate volatile chemical product (VCP; e.g., adhesives, personal care products) emissions in the McDonald et al.
View Article and Find Full Text PDFDespite decades of emission control measures aimed at improving air quality, Los Angeles (LA) continues to experience severe ozone pollution during the summertime. We incorporate cooking volatile organic compound (VOC) emissions in a chemical transport model and evaluate it against observations in order to improve the model representation of the present-day ozone chemical regime in LA. Using this updated model, we investigate the impact of adopting zero-emission vehicles (ZEVs) on ozone pollution with increased confidence.
View Article and Find Full Text PDFEnviron Sci Technol
December 2023
State inventories indicate that dairy operations account for nearly half of California's methane budget. Recent analyses suggest, however, that these emissions may be underestimated, complicating efforts to develop emission reduction strategies. Here, we report estimates of dairy methane emissions in the southern San Joaquin Valley (SJV) of California in June 2021 using airborne flux measurements.
View Article and Find Full Text PDFDrought can affect the capacity of soils to emit and consume biogenic volatile organic compounds (VOCs). Here we show the impact of prolonged drought followed by rewetting and recovery on soil VOC fluxes in an experimental rainforest. Under wet conditions the rainforest soil acts as a net VOC sink, in particular for isoprenoids, carbonyls and alcohols.
View Article and Find Full Text PDFDrought impacts on microbial activity can alter soil carbon fate and lead to the loss of stored carbon to the atmosphere as CO and volatile organic compounds (VOCs). Here we examined drought impacts on carbon allocation by soil microbes in the Biosphere 2 artificial tropical rainforest by tracking C from position-specific C-pyruvate into CO and VOCs in parallel with multi-omics. During drought, efflux of C-enriched acetate, acetone and CHO (diacetyl) increased.
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